HILLIER, James Arthur, PATSALAS, Panos, KARFARIDIS, Dimitrios, CAMELIO, Sophie, CRANTON, Wayne, NABOK, Alexei V., MELLOR, Christopher J., KOUTSOGEORGIS, Demosthenes C. and KALFAGIANNIS, Nikolaos (2022). Photo-engineered optoelectronic properties of indium tin oxide via reactive laser annealing. Scientific Reports, 12 (1): 14986.
Documents
30661:607621
PDF
41598_2022_Article_18883.pdf - Published Version
Available under License Creative Commons Attribution.
41598_2022_Article_18883.pdf - Published Version
Available under License Creative Commons Attribution.
Download (2MB) | Preview
30661:607620
PDF
41598_2022_18883_MOESM1_ESM.pdf - Supplemental Material
Available under License Creative Commons Attribution.
41598_2022_18883_MOESM1_ESM.pdf - Supplemental Material
Available under License Creative Commons Attribution.
Download (2MB) | Preview
Abstract
Abstract: Transparent conductive oxides are appealing materials for optoelectronic and plasmonic applications as, amongst other advantages, their properties can be modulated by engineering their defects. Optimisation of this adjustment is, however, a complex design problem. This work examined the modification of the carrier transport properties of sputtered tin-doped indium oxide (ITO) via laser annealing in reactive environments. We relate the optical modifications to the structural, compositional, and electronic properties to elucidate the precise mechanisms behind the reactive laser annealing (ReLA) process. For sufficiently high laser fluence, we reveal an ambient-dependent and purely compositional modulation of the carrier concentration of ITO thin films. Hereby, we demonstrate that ReLA utilises the precise energy delivery of photonic processing to enhance the carrier mobility and finely tune the carrier concentration without significantly affecting the crystal structure. Exploitation of this phenomena may enable one to selectively engineer the optoelectronic properties of ITO, promising an alternative to the exploration of new materials for optoelectronic and photonic applications.
More Information
Statistics
Downloads
Downloads per month over past year
Downloads per month over past year for
"41598_2022_Article_18883.pdf"
Downloads per month over past year for
"41598_2022_18883_MOESM1_ESM.pdf"
Metrics
Altmetric Badge
Dimensions Badge
Share
Actions (login required)
![]() |
View Item |